Nanocrystal Assemblies: Current Advances and Open Problems (2024)

Bassani, C. L., van Anders, G., Banin, U., Baranov, D., Chen, Q., Dijkstra, M., Dimitriyev, M. S., Efrati, E., Faraudo, J., Gang, O., Gaston, N., Golestanian, R., Guerrero-Garcia, G. I., Gruenwald, M., Haji-Akbari, A., Ibáñez, M., Karg, M., Kraus, T., Lee, B., ... Travesset, A. (2024). Nanocrystal Assemblies: Current Advances and Open Problems. ACS Nano, 18(23), 14791-14840. https://doi.org/10.1021/acsnano.3c10201

Bassani, Carlos L. ; van Anders, Greg ; Banin, Uri et al. / Nanocrystal Assemblies : Current Advances and Open Problems. I: ACS Nano. 2024 ; Vol. 18, Nr. 23. s. 14791-14840.

@article{61c1d0afb0c4438a810c78fcb8d65b7b,

title = "Nanocrystal Assemblies: Current Advances and Open Problems",

abstract = "We explore the potential of nanocrystals (a term used equivalently to nanoparticles) as building blocks for nanomaterials, and the current advances and open challenges for fundamental science developments and applications. Nanocrystal assemblies are inherently multiscale, and the generation of revolutionary material properties requires a precise understanding of the relationship between structure and function, the former being determined by classical effects and the latter often by quantum effects. With an emphasis on theory and computation, we discuss challenges that hamper current assembly strategies and to what extent nanocrystal assemblies represent thermodynamic equilibrium or kinetically trapped metastable states. We also examine dynamic effects and optimization of assembly protocols. Finally, we discuss promising material functions and examples of their realization with nanocrystal assemblies.",

keywords = "assembly protocols, colloidal crystal, material properties, nanocrystal, nanocrystal assembly, nanoparticle, quantum dots, self-assembly, structure prediction, superlattice",

author = "Bassani, {Carlos L.} and {van Anders}, Greg and Uri Banin and Dmitry Baranov and Qian Chen and Marjolein Dijkstra and Dimitriyev, {Michael S.} and Efi Efrati and Jordi Faraudo and Oleg Gang and Nicola Gaston and Ramin Golestanian and Guerrero-Garcia, {G. Ivan} and Michael Gruenwald and Amir Haji-Akbari and Maria Ib{\'a}{\~n}ez and Matthias Karg and Tobias Kraus and Byeongdu Lee and {Van Lehn}, {Reid C.} and Macfarlane, {Robert J.} and Mognetti, {Bortolo M.} and Arash Nikoubashman and Saeed Osat and Prezhdo, {Oleg V.} and Rotskoff, {Grant M.} and Leonor Saiz and An-Chang Shi and Sara Skrabalak and Smalyukh, {Ivan I.} and Mario Tagliazucchi and Talapin, {Dmitri V.} and Tkachenko, {Alexei V.} and Sergei Tretiak and David Vaknin and Asaph Widmer-Cooper and Wong, {Gerard C. L.} and Xingchen Ye and Shan Zhou and Eran Rabani and Michael Engel and Alex Travesset",

note = "Publisher Copyright: {\textcopyright} 2024 American Chemical Society.",

year = "2024",

month = jun,

day = "11",

doi = "10.1021/acsnano.3c10201",

language = "English",

volume = "18",

pages = "14791--14840",

journal = "ACS Nano",

issn = "1936-0851",

publisher = "The American Chemical Society (ACS)",

number = "23",

}

Nanocrystal Assemblies: Current Advances and Open Problems. / Bassani, Carlos L.; van Anders, Greg; Banin, Uri et al.
I: ACS Nano, Vol. 18, Nr. 23, 11.06.2024, s. 14791-14840.

Forskningsoutput: Tidskriftsbidrag › Översiktsartikel › Peer review

TY - JOUR

T1 - Nanocrystal Assemblies

T2 - Current Advances and Open Problems

AU - Bassani, Carlos L.

AU - van Anders, Greg

AU - Banin, Uri

AU - Baranov, Dmitry

AU - Chen, Qian

AU - Dijkstra, Marjolein

AU - Dimitriyev, Michael S.

AU - Efrati, Efi

AU - Faraudo, Jordi

AU - Gang, Oleg

AU - Gaston, Nicola

AU - Golestanian, Ramin

AU - Guerrero-Garcia, G. Ivan

AU - Gruenwald, Michael

AU - Haji-Akbari, Amir

AU - Ibáñez, Maria

AU - Karg, Matthias

AU - Kraus, Tobias

AU - Lee, Byeongdu

AU - Van Lehn, Reid C.

AU - Macfarlane, Robert J.

AU - Mognetti, Bortolo M.

AU - Nikoubashman, Arash

AU - Osat, Saeed

AU - Prezhdo, Oleg V.

AU - Rotskoff, Grant M.

AU - Saiz, Leonor

AU - Shi, An-Chang

AU - Skrabalak, Sara

AU - Smalyukh, Ivan I.

AU - Tagliazucchi, Mario

AU - Talapin, Dmitri V.

AU - Tkachenko, Alexei V.

AU - Tretiak, Sergei

AU - Vaknin, David

AU - Widmer-Cooper, Asaph

AU - Wong, Gerard C. L.

AU - Ye, Xingchen

AU - Zhou, Shan

AU - Rabani, Eran

AU - Engel, Michael

AU - Travesset, Alex

N1 - Publisher Copyright:© 2024 American Chemical Society.

PY - 2024/6/11

Y1 - 2024/6/11

N2 - We explore the potential of nanocrystals (a term used equivalently to nanoparticles) as building blocks for nanomaterials, and the current advances and open challenges for fundamental science developments and applications. Nanocrystal assemblies are inherently multiscale, and the generation of revolutionary material properties requires a precise understanding of the relationship between structure and function, the former being determined by classical effects and the latter often by quantum effects. With an emphasis on theory and computation, we discuss challenges that hamper current assembly strategies and to what extent nanocrystal assemblies represent thermodynamic equilibrium or kinetically trapped metastable states. We also examine dynamic effects and optimization of assembly protocols. Finally, we discuss promising material functions and examples of their realization with nanocrystal assemblies.

AB - We explore the potential of nanocrystals (a term used equivalently to nanoparticles) as building blocks for nanomaterials, and the current advances and open challenges for fundamental science developments and applications. Nanocrystal assemblies are inherently multiscale, and the generation of revolutionary material properties requires a precise understanding of the relationship between structure and function, the former being determined by classical effects and the latter often by quantum effects. With an emphasis on theory and computation, we discuss challenges that hamper current assembly strategies and to what extent nanocrystal assemblies represent thermodynamic equilibrium or kinetically trapped metastable states. We also examine dynamic effects and optimization of assembly protocols. Finally, we discuss promising material functions and examples of their realization with nanocrystal assemblies.

KW - assembly protocols

KW - colloidal crystal

KW - material properties

KW - nanocrystal

KW - nanocrystal assembly

KW - nanoparticle

KW - quantum dots

KW - self-assembly

KW - structure prediction

KW - superlattice

UR - http://www.scopus.com/inward/record.url?scp=85195093044&partnerID=8YFLogxK

U2 - 10.1021/acsnano.3c10201

DO - 10.1021/acsnano.3c10201

M3 - Review article

C2 - 38814908

AN - SCOPUS:85195093044

SN - 1936-0851

VL - 18

SP - 14791

EP - 14840

JO - ACS Nano

JF - ACS Nano

IS - 23

ER -

Bassani CL, van Anders G, Banin U, Baranov D, Chen Q, Dijkstra M et al. Nanocrystal Assemblies: Current Advances and Open Problems. ACS Nano. 2024 juni 11;18(23):14791-14840. Epub 2024 maj 30. doi: 10.1021/acsnano.3c10201